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Funded Research

High-resolution measurements of atmospheric CO2 over North America during NASA Field Campaigns (2004-2008)

Yang, Melissa: NASA Langley Research Center (Project Lead)
Choi, Yonghoon: NASA LaRC/SSAI (Co-Investigator)
Vadrevu, Krishna: NASA MSFC (Co-Investigator)
Woo, Jung-Hun: Konkuk University (Co-Investigator)
Prasad, Narasimha: NASA Langley Research Center (Participant)

Project Funding: 2004 - 2008

Funded by NASA

Abstract:
The Tropospheric Chemistry Program at the National Aeronautics and Space Administration (NASA) has recently conducted a number of airborne science missions over North America and adjacent oceans to understand the impact of long-range transport of trace gases and aerosols on the changing chemical composition of the troposphere. Regional-scale measurements were made over the eastern United States (INTEX-NA summer 2004); Mexico (MILAGRO March 2006); the North Pacific and Alaska (INTEX-B May 2006); the Canadian Arctic (ARCTAS spring and summer 2008); and California (CARB June 2008). For these field campaigns, instrumentation for the in situ measurement of CO2 was integrated on the NASA DC-8 research aircraft providing high-resolution (1 second) data traceable to the global calibration scale. These observations provide unique and definitive data sets via their intermediate-scale coverage, and frequent vertical profiles throughout the troposphere (0.1 – 12 km) for use in inversion and other global modeling studies.

Publications:

Vay, S. A., Tyler, S. C., Choi, Y., Blake, D. R., Blake, N. J., Sachse, G. W., Diskin, G. S., Singh, H. B. 2009. Sources and transport of D<sup>14</sup>C in CO<sub>2</sub> within the Mexico City Basin and vicinity. Atmospheric Chemistry and Physics. 9(14), 4973-4985. DOI: 10.5194/acp-9-4973-2009

Campbell, J. E., Carmichael, G. R., Chai, T., Mena-Carrasco, M., Tang, Y., Blake, D. R., Blake, N. J., Vay, S. A., Collatz, G. J., Baker, I., Berry, J. A., Montzka, S. A., Sweeney, C., Schnoor, J. L., Stanier, C. O. 2008. Photosynthetic Control of Atmospheric Carbonyl Sulfide During the Growing Season. Science. 322(5904), 1085-1088. DOI: 10.1126/science.1164015

Choi, Y., Vay, S. A., Vadrevu, K. P., Soja, A. J., Woo, J., Nolf, S. R., Sachse, G. W., Diskin, G. S., Blake, D. R., Blake, N. J., Singh, H. B., Avery, M. A., Fried, A., Pfister, L., Fuelberg, H. E. 2008. Characteristics of the atmospheric CO2signal as observed over the conterminous United States during INTEX-NA. Journal of Geophysical Research. 113(D7). DOI: 10.1029/2007JD008899

Chahine, M. T., Chen, L., Dimotakis, P., Jiang, X., Li, Q., Olsen, E. T., Pagano, T., Randerson, J., Yung, Y. L. 2008. Satellite remote sounding of mid-tropospheric CO2. Geophysical Research Letters. 35(17). DOI: 10.1029/2008GL035022

Kim, S. Y., Talbot, R., Mao, H., Blake, D., Vay, S., Fuelberg, H. 2008. Continental outflow from the US to the upper troposphere over the North Atlantic during the NASA INTEX-NA Airborne Campaign. Atmospheric Chemistry and Physics. 8(7), 1989-2005. DOI: 10.5194/acp-8-1989-2008

Blake, N. J., Campbell, J. E., Vay, S. A., Fuelberg, H. E., Huey, L. G., Sachse, G., Meinardi, S., Beyersdorf, A., Baker, A., Barletta, B., Midyett, J., Doezema, L., Kamboures, M., McAdams, J., Novak, B., Rowland, F. S., Blake, D. R. 2008. Carbonyl sulfide (OCS): Large-scale distributions over North America during INTEX-NA and relationship to CO2. Journal of Geophysical Research. 113(D9). DOI: 10.1029/2007JD009163

Fried, A., Olson, J. R., Walega, J. G., Crawford, J. H., Chen, G., Weibring, P., Richter, D., Roller, C., Tittel, F., Porter, M., Fuelberg, H., Halland, J., Bertram, T. H., Cohen, R. C., Pickering, K., Heikes, B. G., Snow, J. A., Shen, H., O'Sullivan, D. W., Brune, W. H., Ren, X., Blake, D. R., Blake, N., Sachse, G., Diskin, G. S., Podolske, J., Vay, S. A., Shetter, R. E., Hall, S. R., Anderson, B. E., Thornhill, L., Clarke, A. D., McNaughton, C. S., Singh, H. B., Avery, M. A., Huey, G., Kim, S., Millet, D. B. 2008. Role of convection in redistributing formaldehyde to the upper troposphere over North America and the North Atlantic during the summer 2004 INTEX campaign. Journal of Geophysical Research. 113(D17). DOI: 10.1029/2007JD009760

Talbot, R., Mao, H., Scheuer, E., Dibb, J., Avery, M., Browell, E., Sachse, G., Vay, S., Blake, D., Huey, G., Fuelberg, H. 2008. Factors influencing the large-scale distribution of Hgdeg in the Mexico City area and over the North Pacific. Atmospheric Chemistry and Physics. 8(7), 2103-2114. DOI: 10.5194/acp-8-2103-2008

Bertram, T. H., Perring, A. E., Wooldridge, P. J., Crounse, J. D., Kwan, A. J., Wennberg, P. O., Scheuer, E., Dibb, J., Avery, M., Sachse, G., Vay, S. A., Crawford, J. H., McNaughton, C. S., Clarke, A., Pickering, K. E., Fuelberg, H., Huey, G., Blake, D. R., Singh, H. B., Hall, S. R., Shetter, R. E., Fried, A., Heikes, B. G., Cohen, R. C. 2007. Direct Measurements of the Convective Recycling of the Upper Troposphere. Science. 315(5813), 816-820. DOI: 10.1126/science.1134548

CAMPBELL, J. E., CARMICHAEL, G. R., TANG, Y., CHAI, T., VAY, S. A., CHOI, Y., SACHSE, G. W., SINGH, H. B., SCHNOOR, J. L., WOO, J., VUKOVICH, J. M., STREETS, D. G., HUEY, L. G., STANIER, C. O. 2007. Analysis of anthropogenic CO2signal in ICARTT using a regional chemical transport model and observed tracers. Tellus B. 59(2), 199-210. DOI: 10.1111/j.1600-0889.2006.00239.x

Washenfelder, R. A., Toon, G. C., Blavier, J., Yang, Z., Allen, N. T., Wennberg, P. O., Vay, S. A., Matross, D. M., Daube, B. C. 2006. Carbon dioxide column abundances at the Wisconsin Tall Tower site. Journal of Geophysical Research. 111(D22). DOI: 10.1029/2006JD007154

Palmer, P. I., Suntharalingam, P., Jones, D. B. A., Jacob, D. J., Streets, D. G., Fu, Q., Vay, S. A., Sachse, G. W. 2006. Using CO2:CO correlations to improve inverse analyses of carbon fluxes. Journal of Geophysical Research. 111(D12). DOI: 10.1029/2005JD006697

Lin, J. C., Gerbig, C., Daube, B. C., Wofsy, S. C., Andrews, A. E., Vay, S. A., Anderson, B. E. 2004. An empirical analysis of the spatial variability of atmospheric CO2: Implications for inverse analyses and space-borne sensors. Geophysical Research Letters. 31(23). DOI: 10.1029/2004GL020957

Suntharalingam, P. 2004. Improved quantification of Chinese carbon fluxes using CO2/CO correlations in Asian outflow. Journal of Geophysical Research. 109(D18). DOI: 10.1029/2003JD004362

Vay, S. A. 2003. Influence of regional-scale anthropogenic emissions on CO2distributions over the western North Pacific. Journal of Geophysical Research. 108(D20). DOI: 10.1029/2002JD003094

Vay, S. A., B. E. Anderson, T. J. Conway, G. W. Sachse, J. E. Collins, Jr., D. R. Blake, and D. J. Westberg.1999. Airborne observations of the tropospheric CO2 distribution and its controlling factors over the South Pacific Basin, J. Geophys. Res., 104(D5), 5663-5676.


More details may be found in the following project profile(s):